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Towards chemistry at absolute zero

Abstract:
The prospect of cooling matter down to temperatures that are close to absolute zero raises intriguing questions about how chemical reactivity changes under these extreme conditions. Although some types of chemical reaction still occur at 1 μK, they can no longer adhere to the conventional picture of reactants passing over an activation energy barrier to become products. Indeed, at ultracold temperatures, the system enters a fully quantum regime, and quantum mechanics replaces the classical picture of colliding particles. In this Review, we discuss recent experimental and theoretical developments that allow us to explore chemical reactions at temperatures that range from 100 K to 500 nK. Although the field is still in its infancy, exceptional control has already been demonstrated over reactivity at low temperatures.
Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1038/s41570-020-00239-0

Authors

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Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Physical & Theoretical Chem
Role:
Author
ORCID:
0000-0003-2073-4004


Publisher:
Springer Nature
Journal:
Nature Reviews Chemistry More from this journal
Volume:
5
Pages:
125-140
Publication date:
2021-01-12
Acceptance date:
2020-11-17
DOI:
EISSN:
2397-3358


Language:
English
Keywords:
Pubs id:
1146082
Local pid:
pubs:1146082
Deposit date:
2020-11-19
ARK identifier:

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