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Covariance imaging experiments using a pixel-imaging mass-spectrometry camera

Abstract:
The "pixel imaging mass spectrometry" camera is used to perform femtosecond laser-induced Coulomb explosion imaging of 3,5-dibromo-3′, 5′-difluoro-4′-cyanobiphenyl molecules prealigned in space. The experiment allows the concurrent detection of the correlated two-dimensional momentum images of all the ionic fragments resulting from fragmentation of multiple molecules in each acquisition cycle. The Coulomb explosion studies provide rich information about the parent molecular structure and fragmentation dynamics, and open new opportunities for real-time imaging of intramolecular processes. © 2014 American Physical Society.
Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1103/PhysRevA.89.011401

Authors


More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Physical & Theoretical Chem
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Physical & Theoretical Chem
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Physical & Theoretical Chem
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Physical & Theoretical Chem
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Physical & Theoretical Chem
Role:
Author


More from this funder
Funding agency for:
Vallance, C
Grant:
238671
More from this funder
Funding agency for:
Lauer, A
Grant:
3209/1-1
More from this funder
Funding agency for:
Brouard, M
Vallance, C
Grant:
238671
238671
More from this funder
Funding agency for:
Brouard, M
Vallance, C
Grant:
238671
238671
More from this funder
Funding agency for:
Brouard, M
Vallance, C
Grant:
238671
238671


Publisher:
American Physical Society
Journal:
PHYSICAL REVIEW A More from this journal
Volume:
89
Issue:
1
Publication date:
2014-01-21
DOI:
EISSN:
1094-1622
ISSN:
1050-2947


Language:
English
Pubs id:
pubs:452523
UUID:
uuid:4a7cbf2d-29e1-4592-bee2-6bb32e882919
Local pid:
pubs:452523
Source identifiers:
452523
Deposit date:
2014-05-10

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