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3-Azidoazetidines as the first scaffolds for β-amino azetidine carboxylic acid peptidomimetics: Azetidine iminosugars containing an acetamido group do not inhibit β-N-acetylhexosaminidases

Abstract:
Stable amides and oligopeptides derived from methyl . trans,trans-3-azido-4-hydroxymethyl-l-azetidine carboxylate, prepared in 19% yield from diacetone allose, is the first example of a β-amino-azetidine carboxylic acid incorporated into peptidomimetics and provides a scaffold for investigating secondary structure induced by a novel β-amino acid. A number of azetidine iminosugars containing a NHAc substituent were prepared but none of them were β-N-acetylhexosaminidase inhibitors.
Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1016/j.tetasy.2016.08.001

Authors


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Institution:
University of Oxford
Division:
MSD
Department:
Biochemistry
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Organic Chemistry
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MSD
Department:
Biochemistry
Role:
Author
Publisher:
Elsevier
Journal:
Tetrahedron Asymmetry More from this journal
Volume:
27
Issue:
17-18
Pages:
872-881
Publication date:
2016-08-11
Acceptance date:
2016-08-01
DOI:
EISSN:
1362-511X
ISSN:
0957-4166
Keywords:
Pubs id:
pubs:640539
UUID:
uuid:43d4a69c-9153-4c79-8337-9290cd7c874c
Local pid:
pubs:640539
Source identifiers:
640539
Deposit date:
2016-09-09

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