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A μSR study of the spin-crossover

Abstract:

The spin-crossover phenomenon is a cooperative low-spin to high-spin transition which can be initiated using temperature or light-irradiation. We have used muon-spin relaxation (μSR) to study this effect in Fe(PM-PEA) 2(NCS)2 and Fe(PMAzA)2(NCS)2. We find Gaussian or exponential muon relaxation in the high-spin phase for the two compounds, reflecting differences in their intermolecular interactions. For both compounds, the low-spin phase gives rise to root-exponential relaxation which we asso...

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Publisher copy:
10.1016/j.jpcs.2003.08.017

Authors


Blundell, SJ More by this author
Marshall, IM More by this author
Létard, J-F More by this author
Journal:
Journal of Physics and Chemistry of Solids
Volume:
65
Issue:
1
Pages:
25-28
Publication date:
2004-01-05
DOI:
ISSN:
0022-3697
URN:
uuid:4316fc78-7cfd-4f6c-9150-cc645bc15160
Source identifiers:
344074
Local pid:
pubs:344074
Language:
English

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