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Collective behavior of thermally active colloids

Abstract:
Colloids with patchy metal coating under laser irradiation could act as local heat sources and generate temperature gradients that could induce self-propulsion and interactions between them. The collective behavior of a dilute solution of such thermally active particles is studied using a stochastic formulation. It is found that when the Soret coefficient is positive, the system could be described in a stationary state by the nonlinear Poisson-Boltzmann equation and could adopt density profiles with significant depletion in the middle region when confined. For colloids with a negative Soret coefficient, the system can be described as a dissipative equivalent of a gravitational system. It is shown that in this case the thermally active colloidal solution could undergo an instability at a critical laser intensity, which has similarities to a supernova explosion. © 2012 American Physical Society.

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Publisher copy:
10.1103/PhysRevLett.108.038303

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Journal:
Physical Review Letters More from this journal
Volume:
108
Issue:
3
Publication date:
2012-01-20
DOI:
EISSN:
1079-7114
ISSN:
0031-9007


Language:
English
Pubs id:
pubs:312430
UUID:
uuid:412b38b3-8781-4501-9cd0-965271165aca
Local pid:
pubs:312430
Source identifiers:
312430
Deposit date:
2012-12-19
ARK identifier:

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