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Aerosols enhance cloud lifetime and brightness along the stratus-to-cumulus transition

Abstract:
Anthropogenic aerosols are hypothesized to enhance planetary albedo and offset some of the warming due to the buildup of greenhouse gases in Earth’s atmosphere. Aerosols can enhance the coverage, reflectance, and lifetime of warm low-level clouds. However, the relationship between cloud lifetime and aerosol concentration has been challenging to measure from polar orbiting satellites. We estimate two timescales relating to the formation and persistence of low-level clouds over 1○×1○ spatial domains using multiple years of geostationary satellite observations provided by the Clouds and Earth’s Radiant Energy System (CERES) Synoptic (SYN) product. Lagrangian trajectories spanning several days along the classic stratus-to-cumulus transition zone are stratified by aerosol optical depth and meteorology. Clouds forming in relatively polluted trajectories tend to have lighter precipitation rates, longer average lifetime, and higher cloud albedo and cloud fraction compared with unpolluted trajectories. While liquid water path differences are found to be negligible, we find direct evidence of increased planetary albedo primarily through increased drop concentration (Nd) and cloud fraction, with the caveat that the aerosol influence on cloud fraction is positive only for stable atmospheric conditions. While the increase in cloud fraction can be large typically in the beginning of trajectories, the Twomey effect accounts for the bulk (roughly 3/4) of the total aerosol indirect radiative forcing estimate.
Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1073/pnas.1921231117

Authors

More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Physics
Sub department:
Atmos Ocean & Planet Physics
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Physics
Sub department:
Atmos Ocean & Planet Physics
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Physics
Sub department:
Atmos Ocean & Planet Physics
Oxford college:
Oriel College
Role:
Author
ORCID:
0000-0002-1191-0128


Publisher:
National Academy of Sciences
Journal:
Proceedings of the National Academy of Sciences More from this journal
Volume:
117
Issue:
30
Pages:
17591-17598
Publication date:
2020-07-13
Acceptance date:
2020-06-04
DOI:
EISSN:
1091-6490
ISSN:
0027-8424


Language:
English
Keywords:
Pubs id:
1109341
Local pid:
pubs:1109341
Deposit date:
2020-06-05
ARK identifier:

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