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2-Aminobenzaldehydes as versatile substrates for rhodium-catalyzed alkyne hydroacylation: application to dihydroquinolone synthesis.

Abstract:

Amine for it! A cationic rhodium catalyst, which was assembled insitu from commercial components, promoted the reaction of a range of simple 2-aminobenzaldehydes with terminal and internal alkynes in a series of intermolecular hydroacylation reactions. The products of this reaction, amino-substituted enones, were efficiently converted into the corresponding dihydro-4-quinolones. © 2013 The Authors. Published by Wiley-VCH Verlag GmbH and Co. KGaA. This is an open access article under the terms...

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Publication status:
Published

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Publisher copy:
10.1002/anie.201308127

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Journal:
Angewandte Chemie (International ed. in English)
Volume:
52
Issue:
50
Pages:
13280-13283
Publication date:
2013-12-01
DOI:
EISSN:
1521-3773
ISSN:
1433-7851
Source identifiers:
438779
Language:
English
Keywords:
Pubs id:
pubs:438779
UUID:
uuid:3d6b968c-87c0-4317-97fa-6853daa8c1a6
Local pid:
pubs:438779
Deposit date:
2013-12-12

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