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Filling vacancies in a Prussian blue analogue using mechanochemical post-synthetic modification

Abstract:

Mechanochemical grinding of polycrystalline powders of the Prussian blue analogue (PBA) Mn[Co(CN)6]2/3□1/3·xH2O and K3Co(CN)6 consumes the latter and chemically modifies the former. A combination of inductively-coupled plasma and X-ray powder diffraction measurements suggests the hexacyanometallate vacancy fraction in this modified PBA is reduced by approximately one third under the specific conditions we explore. We infer the mechanochemically-driven incorporation of [Co(CN)6]3− ions onto th...

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Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1039/d0cc02922j

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Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Inorganic Chemistry
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Materials
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Materials
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Materials
Role:
Author
ORCID:
0000-0002-2613-4555
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Inorganic Chemistry
Oxford college:
St Anne's College
Role:
Author
ORCID:
0000-0001-9231-3749
Publisher:
Royal Society of Chemistry Publisher's website
Journal:
Chemical Communications Journal website
Volume:
56
Issue:
57
Pages:
7873-7876
Publication date:
2020-06-04
Acceptance date:
2020-06-04
DOI:
EISSN:
1364-548X
ISSN:
1359-7345
Pmid:
32529992
Language:
English
Keywords:
Pubs id:
1113142
Local pid:
pubs:1113142
Deposit date:
2020-09-29

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