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Electronic temperature driven phase stability and structural evolution of iron at high pressure

Abstract:

We present Gibbs free-energy phase diagrams for compressed iron within a pressure range of 20 to 300 GPa and electronic temperature up to 3 eV obtained using finite-temperature density functional and density functional perturbation theories. Our results for bcc, fcc, and hcp phases predict solid-solid phase transitions in iron driven purely by electronic entropy and temperature. We found a phase transition from hcp to bcc at pressures above 200 GPa, which depends on the electronic temperature. An experimental observation of the stability of the bcc phase above 200 GPa by X-ray Free Electron Laser has recently been reported [1].

Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1103/tm8g-1ld1

Authors

More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Physics
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Physics
Sub department:
Atomic & Laser Physics
Oxford college:
St Peter's College
Role:
Author
ORCID:
0000-0003-1016-0975


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Funder identifier:
https://ror.org/0439y7842
Grant:
EP/W010097/1


Publisher:
American Physical Society
Journal:
Physical Review B More from this journal
Volume:
112
Article number:
134103
Publication date:
2025-10-23
Acceptance date:
2025-10-09
DOI:
EISSN:
2469-9969
ISSN:
2469-9950


Language:
English
Pubs id:
2299630
Local pid:
pubs:2299630
Deposit date:
2025-10-13
ARK identifier:

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