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Muon-spin relaxation investigation of magnetic bistability in a crystalline organic radical compound

Abstract:

We present the results of a muon-spin relaxation (μ+SR) investigation of the crystalline organic radical compound 4-(2-benzimidazolyl)-1,2,3,5-dithiadiazolyl (HbimDTDA), in which we demonstrate the hysteretic magnetic switching of the system that takes place at T=(274 ± 11)K caused by a structural phase transition. Muon-site analysis using electronic structure calculations suggests a range of candidate muon stopping sites. The sites are ...

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Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1016/j.jpcs.2023.111493

Authors


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Institution:
University of Oxford
Division:
MPLS
Department:
Physics
Sub department:
Condensed Matter Physics
Oxford college:
Mansfield College
Role:
Author
ORCID:
0000-0002-3426-0834
Publisher:
Elsevier
Journal:
Journal of Physics and Chemistry of Solids More from this journal
Volume:
181
Article number:
111493
Publication date:
2023-06-15
Acceptance date:
2023-04-19
DOI:
EISSN:
1879-2553
ISSN:
0022-3697
Language:
English
Keywords:
Pubs id:
1494077
Local pid:
pubs:1494077
Deposit date:
2023-11-24

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