Electronic nature of charge density wave and electron-phonon coupling in kagome superconductor KV3Sb5

Journal article

The kagome geometry is an example of frustrated configuration in which rich physics takes place, including the emergence of superconductivity and charge density wave (CDW). Among the kagome metals, ScV$_6$Sn$_6$ hosts an unconventional CDW, with its electronic order showing a different periodicity than that of the phonon which generates it. In this material, a CDW-softened flat phonon band has a second-order collapse at the same time that the first order transition occurs. This phonon band originates from the out-of-plane vibrations of the Sc and Sn atoms, and it is at the base of the electron-phonon-coupling driven CDW phase of ScV$_6$Sn$_6$. Here, we use uniaxial strain to tune the frequency of the flat phonon band, tracking the strain evolution via time-resolved optical spectroscopy and first-principles calculations. Our findings emphasize the capability to induce an enhancement of the unconventional CDW properties in ScV$_6$Sn$_6$ kagome metal through control of strain.Comment: Main text + S

Authors: Luo, H; Gao, Q; Liu, H; Gu, Y; Wu, D

• Publication status: Published
• Peer review status: Peer reviewed
• Publisher: Nature Research
• Journal: Nature Communications
• Volume: 13
• Issue: 1
• Pages: 273-273
• Article number: 273
• Publication date: 2022-01-12
• DOI: 10.1038/s41467-021-27946-6
• EISSN: 2041-1723
• ISSN: 2041-1723
• Language: English
• Keywords: Angle-resolved photoemission spectroscopy; Condensed matter physics; Quantum mechanics; Electronic structure; Band gap; Physics; Fermi surface; Charge density wave; Brillouin zone; Superconductivity; Fermi level; Phonon; Electron