Superconducting nonlinear transport in optically driven high-temperature K3C60

Journal article

Optically driven quantum materials exhibit a variety of non-equilibrium functional phenomena [1-11], which are potentially associated with unique transport properties. However, these transient electrical responses have remained largely unexplored, primarily because of the challenges associated with integrating quantum materials into ultrafast electrical devices. Here, thin films of K3C60 grown by Molecular Beam Epitaxy were connected by coplanar terahertz waveguides to a series of photo-conductive switches. This geometry enabled ultrafast transport measurements at high current densities, providing new information on the photo-induced phase created in the high temperature metal by mid-infrared excitation [12-16]. Nonlinearities in the current-voltage charactersitics of the transient state validate the assignment of transient superconductivity, and point to an inhomogeneous phase in which superconducting regions of the sample are connected by resistive weak links [17-23]. This work opens up the possibility of systematic transport measurements in driven quantum materials, both to probe their properties and to integrate them into ultrafast optoelectronic platforms

Authors: Wang, E; Adelinia, JD; Chavez-Cervantes, M; Matsuyama, T; Fechner, M

• Publication status: Published
• Peer review status: Peer reviewed
• Publisher: Nature Research
• Journal: Nature Communications
• Volume: 14
• Issue: 1
• Pages: 7233-7233
• Article number: 7233
• Publication date: 2023-11-09
• DOI: 10.1038/s41467-023-42989-7
• EISSN: 2041-1723
• ISSN: 2041-1723
• Language: English
• Keywords: Superconductivity; Laser; Condensed matter physics; Transient (computer programming); Optoelectronics; Excited state; Computer science; Materials science; Picosecond; Nonlinear system; Physics; Spectroscopy; Ultrashort pulse; Optics; Voltage; Atomic physics