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Deterministic and robust room-temperature exchange coupling in monodomain multiferroic BiFeO3 heterostructures

Abstract:
Exploiting multiferroic BiFeO3 thin films in spintronic devices requires deterministic and robust control of both internal magnetoelectric coupling in BiFeO3, as well as exchange coupling of its antiferromagnetic order to a ferromagnetic overlayer. Previous reports utilized approaches based on multi-step ferroelectric switching with multiple ferroelectric domains. Because domain walls can be responsible for fatigue, contain localized charges intrinsically or via defects, and present problems for device reproducibility and scaling, an alternative approach using a monodomain magnetoelectric state with single-step switching is desirable. Here we demonstrate room temperature, deterministic and robust, exchange coupling between monodomain BiFeO3 films and Co overlayer that is intrinsic (i.e., not dependent on domain walls). Direct coupling between BiFeO3 antiferromagnetic order and Co magnetization is observed, with ~ 90° in-plane Co moment rotation upon single-step switching that is reproducible for hundreds of cycles. This has important consequences for practical, low power non-volatile magnetoelectric devices utilizing BiFeO3.
Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1038/s41467-017-01581-6

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Role:
Author
ORCID:
0000-0002-4845-7558


Publisher:
Springer Nature
Journal:
Nature Communications More from this journal
Volume:
8
Issue:
1
Pages:
1583
Publication date:
2017-11-17
Acceptance date:
2017-09-27
DOI:
ISSN:
2041-1723
Pmid:
29146896


Language:
English
Keywords:
Pubs id:
pubs:747065
UUID:
uuid:277ea049-f3cf-48c6-b74c-d06c620f448a
Local pid:
pubs:747065
Source identifiers:
747065
Deposit date:
2017-12-07

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