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Probing resonating valence bond states in artificial quantum magnets

Abstract:
Designing and characterizing the many-body behaviors of quantum materials represents a prominent challenge for understanding strongly correlated physics and quantum information processing. We constructed artificial quantum magnets on a surface by using spin-1/2 atoms in a scanning tunneling microscope (STM). These coupled spins feature strong quantum fluctuations due to antiferromagnetic exchange interactions between neighboring atoms. To characterize the resulting collective magnetic states and their energy levels, we performed electron spin resonance on individual atoms within each quantum magnet. This gives atomic-scale access to properties of the exotic quantum many-body states, such as a finite-size realization of a resonating valence bond state. The tunable atomic-scale magnetic field from the STM tip allows us to further characterize and engineer the quantum states. These results open a new avenue to designing and exploring quantum magnets at the atomic scale for applications in spintronics and quantum simulations.
Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1038/s41467-021-21274-5

Authors


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Institution:
University of Oxford
Division:
MPLS
Department:
Physics
Role:
Author


Publisher:
Springer Nature
Journal:
Nature Communications More from this journal
Volume:
12
Article number:
993
Publication date:
2021-02-12
Acceptance date:
2021-01-15
DOI:
ISSN:
2041-1723


Language:
English
Keywords:
Pubs id:
1152595
Local pid:
pubs:1152595
Deposit date:
2021-01-08

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