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Multichannel quantum defect theory (MQDT) analysis of the (2+1 ') mass analyzed threshold ionization (MATI) spectroscopy of NH3

Abstract:

MATI spectra of NH3 have been recorded using two-color (2 + 1′) multiphoton excitation via the B̃ and C̃' states and have been simulated using multichannel quantum defect theory. New vibrational bands in the MATI spectra are reported for intermediate levels up to v2 = 6 in the B̃ state. The spectra obtained should in principle be identical to ZEKE spectra recorded under the same resolution. A good agreement between experiment and theory is obtained by using quantum defects determined previous...

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Publication status:
Published

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Publisher copy:
10.1021/jp003728a

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Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Physical & Theoretical Chem
Role:
Author
Journal:
JOURNAL OF PHYSICAL CHEMISTRY A
Volume:
105
Issue:
23
Pages:
5590-5600
Publication date:
2001-06-14
DOI:
EISSN:
1520-5215
ISSN:
1089-5639
Source identifiers:
172025
Language:
English
Pubs id:
pubs:172025
UUID:
uuid:1b432220-7f27-4ede-b980-c7480a8287e6
Local pid:
pubs:172025
Deposit date:
2013-11-16

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