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THz carrier dynamics and magnetotransport study of topological surface states in thin film Bi2Se3

Abstract:
The surface of a topological insulator harbors exotic topological states, protected against backscattering from disorder by time reversal symmetry. The study of these exotic quantum states not only provides an opportunity to explore fundamental phenomena in condensed matter physics, such as the spin Hall effect, but also lays the foundation for applications from quantum computing to spintronics. Conventional electrical measurements suffer from substantial bulk interference, making it difficult to clearly distinguish topological surface states from bulk states. Employing terahertz time-domain spectroscopy, we study the temperature-dependent optical behavior of a 23-quintuple-thick film of bismuth selenide (Bi2Se3) allowing for the deconvolution of the surface state response from the bulk. Our measurement of carrier dynamics give an optical mobility exceeding 2100 cm2/V•s at 4 K, indicative of a surface-dominated response, and a scattering lifetime of ~0.18 ps and a carrier density of 6×1012 cm-2 at 4 K for the Bi2Se3 film. The sample was further processed into a Hall bar device using two different etching techniques, a wet chemical etching and Ar+ ion milling, which resulting in a reduced Hall mobility. Even so, the magneto-conductance transport reveals weak antilocalization behavior in our Bi2Se3 sample, consistent with the presence of a single topological surface state mode.
Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1117/12.2289116

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Institution:
University of Oxford
Division:
Maths, Physical & Life Sciences
Department:
Physics; Condensed Matter Physics
Role:
Author


Publisher:
Society of Photo-Optical Instrumentation Engineers
Host title:
Proceedings of SPIE - The International Society for Optical Engineering
Journal:
Proceedings of SPIE - The International Society for Optical Engineering More from this journal
Volume:
10531
Publication date:
2018-02-23
Acceptance date:
2018-02-23
Event location:
San Francicsco, USA
DOI:
EISSN:
1996-756X
ISSN:
0277-786X
ISBN:
9781510615472


Pubs id:
pubs:859761
UUID:
uuid:19c5ff86-276c-4e09-8205-5d516d889fd4
Local pid:
pubs:859761
Source identifiers:
859761
Deposit date:
2018-06-30

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