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Coarse and fine-tuning of lasing transverse electromagnetic modes in coupled all-inorganic perovskite quantum dots

Abstract:
Inorganic perovskite lasers are of particular interest, with much recent work focusing on Fabry-Pérot cavity-forming nanowires. We demonstrate the direct observation of lasing from transverse electromagnetic (TEM) modes with a long coherence time ∼ 9.5 ps in coupled CsPbBr3 quantum dots, which dispense with an external cavity resonator and show how the wavelength of the modes can be controlled via two independent tuning-mechanisms. Controlling the pump power allowed us to fine-tune the TEM mode structure to the emission wavelength, thus providing a degree of control over the properties of the lasing signal. The temperature-tuning provided an additional degree of control over the wavelength of the lasing peak, importantly, maintained a constant full width at half maximum (FWHM) over the entire tuning range without mode-hopping.
Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1007/s12274-020-3051-y

Authors


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Institution:
University of Oxford
Division:
MPLS
Department:
Physics
Sub department:
Condensed Matter Physics
Role:
Author
ORCID:
0000-0002-5960-3522
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Physics
Sub department:
Condensed Matter Physics
Role:
Author
ORCID:
0000-0002-0507-6579
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Physics
Sub department:
Condensed Matter Physics
Role:
Author
ORCID:
0000-0002-7785-1968


Publisher:
Springer
Journal:
Nano Research More from this journal
Volume:
14
Pages:
108-113
Publication date:
2020-09-12
Acceptance date:
2020-08-11
DOI:
EISSN:
1998-0000
ISSN:
1998-0124


Language:
English
Keywords:
Pubs id:
1132624
Local pid:
pubs:1132624
Deposit date:
2020-09-17

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