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EPR OF SPIN-CORRELATED RADICAL PAIRS - ANALYTICAL TREATMENT OF SELECTIVE EXCITATION INCLUDING ZERO-QUANTUM COHERENCE

Abstract:

We present a simple analytical treatment of the electron paramagnetic resonance (EPR) spectra of spin-correlated radical pairs, including the zero-quantum coherence with which they are created. We concentrate on the time dependence of the spectrum of a prototype radical pair, with exchange and dipolar couplings but no nuclei, in transient nutation experiments with a without a delay between the formation of the pair and the application of the microwave field. We show how the zero-quantum coher...

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Publication status:
Published

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Institution:
University of Oxford
Department:
Oxford, MPLS, Chemistry, Physical and Theoretical Chem
Role:
Author
Journal:
CHEMICAL PHYSICS LETTERS
Volume:
203
Issue:
1
Pages:
65-74
Publication date:
1993-02-12
DOI:
ISSN:
0009-2614
URN:
uuid:14ac57b9-804a-4908-aaec-4f4070cc9f7a
Source identifiers:
44034
Local pid:
pubs:44034

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