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Product spin-orbit state resolved dynamics of the H+H2O and H+D2O abstraction reactions.

Abstract:

The product state-resolved dynamics of the reactions H+H(2)O/D(2)O-->OH/OD((2)Pi(Omega);v',N',f )+H(2)/HD have been explored at center-of-mass collision energies around 1.2, 1.4, and 2.5 eV. The experiments employ pulsed laser photolysis coupled with polarized Doppler-resolved laser induced fluorescence detection of the OH/OD radical products. The populations in the OH spin-orbit states at a collision energy of 1.2 eV have been determined for the H+H(2)O reaction, and for low rotational le...

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Publication status:
Published

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Publisher copy:
10.1063/1.1809578

Authors


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Institution:
University of Oxford
Department:
Oxford, MPLS, Chemistry, Physical and Theoretical Chem
Marinakis, S More by this author
Rubio Lago, L More by this author
Tampkins, P More by this author
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Journal:
The Journal of chemical physics
Volume:
121
Issue:
21
Pages:
10426-10436
Publication date:
2004-12-05
DOI:
EISSN:
1089-7690
ISSN:
0021-9606
URN:
uuid:14526a94-a0f8-4367-8cd6-62b2eedea98e
Source identifiers:
32916
Local pid:
pubs:32916
Language:
English

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