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Bimolecular recombination in methylammonium lead triiodide perovskite is an inverse absorption process

Abstract:

Photovoltaic devices based on metal halide perovskites are rapidly improving in efficiency. Once the Shockley–Queisser limit is reached, charge-carrier extraction will be limited only by radiative bimolecular recombination of electrons with holes. Yet, this fundamental process, and its link with material stoichiometry, is still poorly understood. Here we show that bimolecular charge-carrier recombination in methylammonium lead triiodide perovskite can be fully explained as the inverse process...

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Publication status:
Published
Peer review status:
Peer reviewed
Version:
Publisher's version

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Publisher copy:
10.1038/s41467-017-02670-2

Authors


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Institution:
University of Oxford
Division:
MPLS Division
Department:
Physics
More by this author
Institution:
University of Oxford
Division:
MPLS Division
Department:
Physics
ORCID:
0000-0003-2925-172X
More by this author
Institution:
University of Oxford
Division:
MPLS Division
Department:
Physics
More by this author
Institution:
University of Oxford
Division:
MPLS Division
Department:
Physics
More by this author
Institution:
University of Oxford
Division:
MPLS Division
Department:
Engineering Science
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Grant:
EP/L024667/1, EP/P006329/1, EP/P033229/1, M0205171/1
Publisher:
Springer Nature Publisher's website
Journal:
Nature Communications Journal website
Volume:
9
Pages:
Article: 293
Publication date:
2018-01-18
Acceptance date:
2017-12-15
DOI:
EISSN:
2041-1723
ISSN:
2041-1723
Pubs id:
pubs:821058
URN:
uri:138af7dc-9c0f-432d-b54f-bd35b3c23be6
UUID:
uuid:138af7dc-9c0f-432d-b54f-bd35b3c23be6
Local pid:
pubs:821058
Language:
English
Keywords:

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