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Enhanced photosusceptibility near Tc for the light-induced insulator-to-metal phase transition in vanadium dioxide.

Abstract:
We use optical-pump terahertz-probe spectroscopy to investigate the near-threshold behavior of the photoinduced insulator-to-metal (IM) transition in vanadium dioxide thin films. Upon approaching Tc a reduction in the fluence required to drive the IM transition is observed, consistent with a softening of the insulating state due to an increasing metallic volume fraction (below the percolation limit). This phase coexistence facilitates the growth of a homogeneous metallic conducting phase following superheating via photoexcitation. A simple dynamic model using Bruggeman effective medium theory describes the observed initial condition sensitivity.
Publication status:
Published

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Publisher copy:
10.1103/physrevlett.99.226401

Authors


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Institution:
University of Oxford
Division:
MPLS
Department:
Physics
Sub department:
Atomic & Laser Physics
Role:
Author


Journal:
Physical Review Letters More from this journal
Volume:
99
Issue:
22
Pages:
226401
Publication date:
2007-11-01
DOI:
EISSN:
1079-7114
ISSN:
0031-9007


Language:
English
Pubs id:
pubs:14152
UUID:
uuid:125ed3ca-254f-4773-ac06-aacd7aed1e9a
Local pid:
pubs:14152
Source identifiers:
14152
Deposit date:
2012-12-19

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