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Edge-enriched 2D MoS 2 thin films grown by chemical vapor deposition for enhanced catalytic performance

Abstract:

Chemical vapor deposition (CVD) is used to grow thin films of 2D MoS2 with nanostructure for catalytic applications in the hydrogen evolution reaction (HER). Tailoring of the CVD parameters results in an optimized MoS2 structure for the HER that consists of large MoS2 platelets with smaller layered MoS2 sheets growing off it in a perpendicular direction, which increases the total number of edge sites within a given geometric area. A surface area to geometric area ratio of up to ∼340 is achiev...

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Publication status:
Published
Peer review status:
Peer reviewed
Version:
Accepted manuscript

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Publisher copy:
10.1021/acscatal.6b02663

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Institution:
University of Oxford
Department:
Wolfson College
More by this author
Institution:
University of Oxford
Department:
Oxford, MPLS, Materials
More by this author
Institution:
University of Oxford
Department:
Oxford, MPLS, Materials
More by this author
Institution:
University of Oxford
Department:
Oxford, MPLS, Materials
More by this author
Institution:
University of Oxford
Department:
Oxford, MPLS, Chemistry
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Publisher:
American Chemical Society Publisher's website
Journal:
ACS Catalysis Journal website
Volume:
7
Issue:
1
Pages:
877-886
Publication date:
2016-12-27
Acceptance date:
2016
DOI:
EISSN:
2155-5435
ISSN:
2155-5435
Pubs id:
pubs:677381
URN:
uri:0fb634f3-dc55-470e-8e14-48111aef1cd0
UUID:
uuid:0fb634f3-dc55-470e-8e14-48111aef1cd0
Local pid:
pubs:677381

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