Journal article icon

Journal article

Characterizing heterogeneous dynamics at hydrated electrode surfaces.

Abstract:

In models of Pt 111 and Pt 100 surfaces in water, motions of molecules in the first hydration layer are spatially and temporally correlated. To interpret these collective motions, we apply quantitative measures of dynamic heterogeneity that are standard tools for considering glassy systems. Specifically, we carry out an analysis in terms of mobility fields and distributions of persistence times and exchange times. In so doing, we show that dynamics in these systems is facilitated by transient...

Expand abstract
Publication status:
Published

Actions


Access Document


Publisher copy:
10.1063/1.4803503

Authors


More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Materials
Role:
Author
Journal:
Journal of chemical physics
Volume:
138
Issue:
18
Pages:
184702
Publication date:
2013-05-01
DOI:
EISSN:
1089-7690
ISSN:
0021-9606
Source identifiers:
406667
Language:
English
Pubs id:
pubs:406667
UUID:
uuid:0f3373f0-380f-40d2-8b7c-0a9d65627816
Local pid:
pubs:406667
Deposit date:
2013-11-16

Terms of use


Views and Downloads






If you are the owner of this record, you can report an update to it here: Report update to this record

TO TOP