- Abstract:
-
In models of Pt 111 and Pt 100 surfaces in water, motions of molecules in the first hydration layer are spatially and temporally correlated. To interpret these collective motions, we apply quantitative measures of dynamic heterogeneity that are standard tools for considering glassy systems. Specifically, we carry out an analysis in terms of mobility fields and distributions of persistence times and exchange times. In so doing, we show that dynamics in these systems is facilitated by transient...
Expand abstract - Publication status:
- Published
- Publisher copy:
- 10.1063/1.4803503
-
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- Journal:
- The Journal of chemical physics
- Volume:
- 138
- Issue:
- 18
- Pages:
- 184702
- Publication date:
- 2013-05-05
- DOI:
- EISSN:
-
1089-7690
- ISSN:
-
0021-9606
- URN:
-
uuid:0f3373f0-380f-40d2-8b7c-0a9d65627816
- Source identifiers:
-
406667
- Local pid:
- pubs:406667
- Language:
- English
- Copyright date:
- 2013
Journal article
Characterizing heterogeneous dynamics at hydrated electrode surfaces.
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