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Evidence for unidirectional nematic bond ordering in FeSe

Abstract:
The lifting of $d_{xz}$-$d_{yz}$ orbital degeneracy is often considered a hallmark of the nematic phase of Fe-based superconductors, including FeSe, but its origin is not yet understood. Here we report a high resolution Angle-Resolved Photoemission Spectroscopy study of single crystals of FeSe, accounting for the photon-energy dependence and making a detailed analysis of the temperature dependence. We find that the hole pocket undergoes a fourfold-symmetry-breaking distortion in the nematic phase below 90~K, but in contrast the changes to the electron pockets do not require fourfold symmetry-breaking. Instead, there is an additional separation of the existing $d_{xy}$ and $d_{xz/yz}$ bands - which themselves are not split within resolution. These observations lead us to propose a new scenario of "unidirectional nematic bond ordering" to describe the low-temperature electronic structure of FeSe, supported by a good agreement with 10-orbital tight binding model calculations.
Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1103/PhysRevB.94.201107

Authors



More from this funder
Funding agency for:
Haghighirad, A
Grant:
EP/M020517/1
More from this funder
Funding agency for:
Coldea, A
Grant:
Career Acceleration Fellowship (EP/I004475/1
EP/L001772/1,EP/I004475/1,EP/I017836/1


Publisher:
American Physical Society
Journal:
Physical Review B More from this journal
Volume:
94
Pages:
201107(R)
Publication date:
2016-01-01
Acceptance date:
2016-10-04
DOI:
EISSN:
2469-9969
ISSN:
2469-9950


Keywords:
Pubs id:
pubs:612164
UUID:
uuid:0e7b85fd-ba41-4dbb-be59-496c347098ea
Local pid:
pubs:612164
Source identifiers:
612164
Deposit date:
2016-10-13

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