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Spin-orbit coupled spin-polarised hole gas at the CrSe2-terminated surface of AgCrSe2

Abstract:

In half-metallic systems, electronic conduction is mediated by a single spin species, offering enormous potential for spintronic devices. Here, using microscopic-area angle-resolved photoemission, we show that a spin-polarised two-dimensional hole gas is naturally realised in the polar magnetic semiconductor AgCrSe2 by an intrinsic self-doping at its CrSe2-terminated surface. Through comparison with first-principles calculations, we unveil a striking role of spin-orbit coupling for the surface hole gas, unlocked by both bulk and surface inversion symmetry breaking, suggesting routes for stabilising complex magnetic textures in the surface layer of AgCrSe2.

Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1038/s41535-023-00593-4

Authors



Publisher:
Springer Nature
Journal:
npj Quantum Materials More from this journal
Volume:
8
Article number:
61
Publication date:
2023-10-21
Acceptance date:
2023-10-09
DOI:
EISSN:
2397-4648


Language:
English
Keywords:
Pubs id:
1552856
Local pid:
pubs:1552856
Deposit date:
2023-10-27

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