- Abstract:
-
A detailed simulation of Fourier transformed large amplitude square-wave voltammetry is presented in the frequency domain for the process Red ⇌ Ox + e-. The simulation takes into account the influence of the electrode kinetics (Butler-Volmer model), uncompensated resistance (R u) and double layer capacitance (Cdl). Of particular significance is the prediction that the even harmonic responses are only detected in the presence of quasi-reversibility or uncompensated resistance, and also are ess...
Expand abstract - Publication status:
- Published
- Publisher copy:
- 10.1002/elan.200403293
-
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- Journal:
- ELECTROANALYSIS
- Volume:
- 17
- Issue:
- 15-16
- Pages:
- 1450-1462
- Publication date:
- 2005-08-05
- DOI:
- EISSN:
-
1521-4109
- ISSN:
-
1040-0397
- URN:
-
uuid:0e12eb83-4bc4-4c24-9bb5-e571d2a71c04
- Source identifiers:
-
131851
- Local pid:
- pubs:131851
- Copyright date:
- 2005
Journal article
Fourier transformed large amplitude square-wave voltammetry as an alternative to impedance spectroscopy: Evaluation of resistance, capacitance and electrode kinetic effects via an heuristic approach
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