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Dependence of line shapes in femtosecond broadband stimulated Raman spectroscopy on pump-probe time delay.

Abstract:

The effect of the time delay between the picosecond Raman pump and the femtosecond Stokes probe pulse on the Raman gain line shape in femtosecond broadband stimulated Raman spectroscopy (FSRS) is presented. Experimental data are obtained for cyclohexane to investigate the dependence of the FSRS line shape on this time delay. Theoretical simulations of the line shapes as a function of the time delay using the coupled wave theory agree well with experimental data, recovering broad line shapes a...

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Publication status:
Published

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Publisher copy:
10.1063/1.1828044

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Institution:
University of Oxford
Department:
Oxford, MPLS, Chemistry, Physical and Theoretical Chem
Role:
Author
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Journal:
The Journal of chemical physics
Volume:
122
Issue:
2
Pages:
024505
Publication date:
2005-01-05
DOI:
EISSN:
1089-7690
ISSN:
0021-9606
URN:
uuid:06e12f52-79a0-452d-a353-b1bfdb76310e
Source identifiers:
118459
Local pid:
pubs:118459
Language:
English

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