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Highly functionalized cyclic and bicyclic β−amino acids from sugar β−nitroesters

Abstract:
The synthesis of highly functionalized bicyclic and cyclic β-amino acids from β-nitrosugars is reported. Specifically, our strategy for the synthesis of polyhydroxylated cyclopentane β-amino acids via the intramolecular C-alkylation of 6-nitro-2-O-triflates of furanosides has been applied to the preparation of the first two examples of a novel class of bicyclic β-amino acids and a novel cyclopentene β-amino acid. Also, our Henry reaction mediated strategy for the synthesis of polyhydroxylated cyclohexane β-amino acids has been extended to a divergent, stereoselective synthesis of new polysubstituted cyclohexane and cyclopentane β-amino acids.
Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1016/j.tet.2019.130837

Authors


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Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Organic Chemistry
Role:
Author
ORCID:
0000-0003-1903-270X


Publisher:
Elsevier
Journal:
Tetrahedron More from this journal
Volume:
76
Issue:
3
Article number:
130837
Publication date:
2019-11-28
Acceptance date:
2019-11-26
DOI:
EISSN:
1464-5416
ISSN:
0040-4020


Language:
English
Keywords:
Pubs id:
pubs:1079754
UUID:
uuid:fdb52de6-b09d-4afa-964f-48c277e7bab6
Local pid:
pubs:1079754
Source identifiers:
1079754
Deposit date:
2019-12-26

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