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Overpotential from cosolvent imbalance in battery electrolytes: LiPF6 in EMC:EC

Abstract:

Most liquid lithium-ion-battery electrolytes incorporate cosolvent blends, but the dominant electrochemical transport models adopt a single-solvent approximation, which assumes in part that nonuniform cosolvent ratios do not affect cell voltage. For the popular electrolyte formulation based on ethyl-methyl carbonate (EMC), ethylene carbonate (EC), and LiPF6, we perform measurements with fixed-reference concentration cells, finding appreciable liquid-junction potentials when only th...

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Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1021/acsomega.3c02088

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More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Engineering Science
Research group:
The Faraday Institution
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Engineering Science
Research group:
The Faraday Institution
Role:
Author
ORCID:
0000-0002-9894-5023
Publisher:
American Chemical Society
Journal:
ACS Omega More from this journal
Volume:
8
Issue:
23
Pages:
21133–21144
Publication date:
2023-05-26
Acceptance date:
2023-05-09
DOI:
EISSN:
2470-1343
Language:
English
Keywords:
Subjects:
Pubs id:
1354634
Local pid:
pubs:1354634
Deposit date:
2023-06-09

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