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Quantitative differences in sulfur poisoning phenomena over ruthenium and palladium: An attempt to deconvolute geometric and electronic poisoning effects using model catalysts

Abstract:

Sulfur poisoning over noble-metal catalysts has traditionally been regarded as very complex and precluding from easy rational understanding, because of the problems of interference from using different supports, inability of controlling coverage due to nonuniform metal particle size, intrinsic size/shape effect of metal component, etc. Here, high-quality polyvinylpyrrolidone (PVP) polymer-supported ruthenium and palladium model nanocatalysts using without solid support are equivalently modifi...

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Publication status:
Published
Peer review status:
Peer reviewed
Version:
Accepted manuscript

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Publisher copy:
10.1021/acscatal.6b02765

Authors


Cookson, J More by this author
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Engineering and Physical Sciences Research Council More from this funder
Johnson Matthey More from this funder
Oxford University More from this funder
Publisher:
American Chemical Society Publisher's website
Journal:
ACS Catalysis Journal website
Volume:
7
Issue:
1
Pages:
592-605
Publication date:
2016-12-05
Acceptance date:
2016-11-26
DOI:
EISSN:
2155-5435
ISSN:
2155-5435
Pubs id:
pubs:698750
URN:
uri:ef7b06c1-90b6-435d-9dee-daa8e306908b
UUID:
uuid:ef7b06c1-90b6-435d-9dee-daa8e306908b
Local pid:
pubs:698750

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