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Synthesis and characterization of [Ru@Ge12]3-: an endohedral 3-connected cluster

Abstract:
The 12-vertex endohedral cluster [Ru@Ge12](3-) reveals an unprecedented D2d-symmetric 3-connected polyhedral geometry. The structure contrasts dramatically with the known deltahedral or approximately deltahedral geometries of [M@Pb12](2-) (M = Ni, Pd, Pt) and [Mn@Pb12](3-) and is a result of extensive delocalization of electron density from the transition-metal center onto the cage.
Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1021/ja411280v

Authors


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Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Inorganic Chemistry
Role:
Author
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Department:
CHEMISTRY
Sub department:
Inorganic Chemistry
Role:
Author
ORCID:
0000-0001-5935-9112
More by this author
Department:
CHEMISTRY
Sub department:
Inorganic Chemistry
Role:
Author
ORCID:
0000-0002-8991-1921
More by this author
Department:
CHEMISTRY
Sub department:
Inorganic Chemistry
Role:
Author
ORCID:
0000-0002-7311-1663


More from this funder
Grant:
EP/D048559/1
EP/F00186X/1
EP/L011972/1
EP/K021435/1


Publisher:
American Chemical Society
Journal:
Journal of the American Chemical Society More from this journal
Volume:
136
Issue:
4
Pages:
1210-1213
Place of publication:
United States
Publication date:
2014-01-14
Acceptance date:
2013-12-30
DOI:
EISSN:
1520-5126
ISSN:
0002-7863
Pmid:
24377744


Language:
English
Keywords:
Pubs id:
445536
Local pid:
pubs:445536
Deposit date:
2020-07-30

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