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Glycerol hydrogenolysis over a Pt-Ni bimetallic catalyst with hydrogen generated in situ

Abstract:

Using hydrogen generated in situ from aqueous phase reforming provides an efficient and economic route for glycerol hydrogenolysis. A Pt-Ni bimetallic catalyst supported on γ-Al 2 O 3 has been prepared to catalyze the selective hydrogenolysis of glycerol to 1,2-propanediol, with glycerol conversion reaching 71.4% in 3 h. The significant promotion of conversion and selectivity could be explained by the formation of Pt-Ni alloy based on catalyst characterization. The effects of Pt/Ni ratio, re...

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Publication status:
Published
Peer review status:
Peer reviewed
Version:
Publisher's version

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Publisher copy:
10.1039/c7ra05814d

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Institution:
University of Oxford
Division:
MPLS Division
Department:
Chemistry; Inorganic Chemistry
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MPLS Division
Department:
Chemistry; Inorganic Chemistry
Oxford college:
St Catherines College
Role:
Author
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National Natural Science Foundation of China More from this funder
Fundamental Research Funds for the Central Universities More from this funder
China Scholarship Council More from this funder
Publisher:
Royal Society of Chemistry Publisher's website
Journal:
RSC Advances Journal website
Volume:
7
Issue:
61
Pages:
38251-38256
Publication date:
2017-08-05
Acceptance date:
2017-07-12
DOI:
EISSN:
2046-2069
Pubs id:
pubs:723913
URN:
uri:ea9a91eb-7ecf-435e-b67e-950b69add06d
UUID:
uuid:ea9a91eb-7ecf-435e-b67e-950b69add06d
Local pid:
pubs:723913
Keywords:

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