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Coulomb-explosion imaging using a pixel-imaging mass-spectrometry camera

Abstract:

Femtosecond laser-induced Coulomb-explosion imaging of 3,5-dibromo-3′,5′-difluoro-4′-cyanobiphenyl molecules prealigned in space is explored using a pixel-imaging mass-spectrometry (PImMS) camera. The fast-event-triggered camera allows the concurrent detection of the correlated two-dimensional momentum images, or covariance maps, of all the ionic fragments resulting from fragmentation of multiple molecules in each acquisition cycle. Detailed simulation of the covariance maps reveals that they...

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Publication status:
Published
Peer review status:
Peer reviewed

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Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Physical & Theoretical Chem
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Physical & Theoretical Chem
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Physical & Theoretical Chem
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Physical & Theoretical Chem
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Chemistry Research Laboratory
Role:
Author
More from this funder
Name:
ISIS Innovation Ltd
Funding agency for:
Brouard, M
Vallance, C
Grant:
ST/J002895/1
ST/J002895/1
More from this funder
Name:
Deutsche Forschungsgemeinschaft
Funding agency for:
Lauer, A
Grant:
LA 3209/1-2
More from this funder
Name:
Science and Technology Facilities Council
Funding agency for:
Brouard, M
Vallance, C
Grant:
ST/J002895/1
ST/J002895/1
More from this funder
Name:
European Union
Funding agency for:
Brouard, M
Vallance, C
Grant:
ST/J002895/1
ST/J002895/1
More from this funder
Name:
Engineering and Physical Sciences Research Council
Funding agency for:
Brouard, M
Vallance, C
Grant:
ST/J002895/1
ST/J002895/1
Publisher:
American Physical Society
Journal:
Physical Review A More from this journal
Volume:
91
Issue:
5
Article number:
053424
Publication date:
2015-05-28
DOI:
EISSN:
1094-1622
ISSN:
1050-2947
Pubs id:
pubs:527510
UUID:
uuid:e762e029-2479-43da-891d-c7e299335a66
Local pid:
pubs:527510
Source identifiers:
527510
Deposit date:
2015-06-24

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