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Thesis

Towards the total synthesis of calyciphylline A-type Daphniphyllum alkaloids

Abstract:

This thesis details the studies towards the total synthesis of the calyciphylline A-type Daphniphyllum alkaloids, with a particular focus on daphniyunnine D (23).

Chapter 1 introduces these biologically and synthetically interesting polycyclic natural products and describes our designed approach towards their synthesis. Separate studies targeting the construction of two tricyclic ring systems have been developed. These provide rapid entry to synthetically versatile intermed...

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Institution:
University of Oxford
Research group:
Professor Darren J. Dixon
Oxford college:
St Hugh's College
Department:
Mathematical,Physical & Life Sciences Division - Chemistry - Organic Chemistry

Contributors

Role:
Supervisor
Publication date:
2014
Type of award:
DPhil
Level of award:
Doctoral
Awarding institution:
Oxford University, UK
URN:
uuid:e506466b-5954-4245-babe-f7bdc6a022c2
Local pid:
ora:9177

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