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Particle-electrode impacts: Evidencing partial versus complete oxidation via variable temperature studies

Abstract:

The partial electro-oxidation of large silver nanoparticles is evidenced by comparing the charges passed in nanoparticle-electrode impacts at a range of temperatures. For larger silver nanoparticles (>100 nm diameter), the variation in the charge passed per nano-impact event at higher temperatures demonstrates that single nanoparticles undergo multiple oxidations events at the electrode, and these oxidations do not go to completion. In contrast, the relative insensitivity of the charge pas...

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Publication status:
Published
Peer review status:
Peer reviewed
Version:
Accepted Manuscript

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Publisher copy:
10.1016/j.jelechem.2018.06.050

Authors


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Institution:
University of Oxford
Division:
MPLS Division
Department:
Chemistry; Physical and Theoretical Chemistry
More by this author
Institution:
University of Oxford
Division:
MPLS Division
Department:
Chemistry; Physical and Theoretical Chemistry
More by this author
Institution:
University of Oxford
Division:
MPLS Division
Department:
Chemistry; Physical and Theoretical Chemistry
More by this author
Institution:
University of Oxford
Division:
Maths, Physical & Life Sciences
Department:
Materials
More by this author
Institution:
University of Oxford
Division:
MPLS Division
Department:
Chemistry; Physical and Theoretical Chemistry
Oxford college:
St John's College
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Grant:
Seventh Framework Programme: 320403
Publisher:
Elsevier Publisher's website
Journal:
Journal of Electroanalytical Chemistry Journal website
Volume:
823
Pages:
492-498
Publication date:
2018-07-03
Acceptance date:
2018-06-27
DOI:
EISSN:
1873-2569
ISSN:
1572-6657
Pubs id:
pubs:870153
URN:
uri:e3fa77bf-8d24-4be2-a183-3d0a5eb4903e
UUID:
uuid:e3fa77bf-8d24-4be2-a183-3d0a5eb4903e
Local pid:
pubs:870153

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