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Rhodium-catalysed intermolecular alkyne hydroacylation: the enantioselective synthesis of α- and β-substituted ketones by kinetic resolution.

Abstract:
Chemical Equation Presented Cleared up! Intermolecular alkyne hydroacylation represents a new addition to the range of transition- metalcatalysed hydroacylation reactions that can be performed in an enantioselective manner. By using a kinetic resolution procedure, both racemic α- and βsubstituted aldehydes can be converted into the corresponding enantiomerically enriched substituted enone products (see scheme). © 2010 Wiley-VCH Verlag GmbH and Co. KGaA, Weinheim.
Publication status:
Published

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Publisher copy:
10.1002/chem.201001748

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Institution:
University of Oxford
Department:
Oxford, MPLS, Chemistry, Inorganic Chemistry
Role:
Author
Journal:
Chemistry (Weinheim an der Bergstrasse, Germany)
Volume:
16
Issue:
36
Pages:
10950-10954
Publication date:
2010-09-05
DOI:
EISSN:
1521-3765
ISSN:
0947-6539
URN:
uuid:dfe2179a-3726-43d2-a31a-9c4d64cbfec0
Source identifiers:
67467
Local pid:
pubs:67467

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