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ROTATIONAL AUTOIONIZATION DYNAMICS IN HIGH RYDBERG STATES OF NITROGEN

Abstract:

The decay dynamics of the high Rydberg states of N2 converging on the first few rotational levels (N+ = 0,1,2,3) of the ground vibronic X 2Σg+ (v+ = 0) state of the N2+ cation have been investigated by delayed pulsed field ionization (PFI) following two-photon enhanced (2+1′) three-photon excitation via the a″ 1Σg+ (v′ = 0) state of N2. The experiments were carried out in the presence of a weak homogeneous dc electric field and at typical ion densities of 200-2000 ions/mm3. All Rydberg states...

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Publication status:
Published

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Publisher copy:
10.1063/1.470639

Authors


MACKENZIE, S More by this author
SOFTLEY, T More by this author
Journal:
JOURNAL OF CHEMICAL PHYSICS
Volume:
103
Issue:
11
Pages:
4509-4518
Publication date:
1995-09-15
DOI:
ISSN:
0021-9606
URN:
uuid:d6e5750c-096c-429b-bc54-9b5649e89339
Source identifiers:
44946
Local pid:
pubs:44946
Language:
English

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