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Iridium-catalyzed C4-alkylation of 2,6-di-tert-butylphenol by using hydrogen-borrowing catalysis

Abstract:
An iridium-catalyzed hydrogen borrowing process has been developed whereby 2,6-di-tert-butylphenol can be alkylated at the C4-position using a range of different primary alcohols (11 examples, 40–93% yield). Following this, a selection of the products obtained underwent retroFriedel–Crafts reaction to provide para-substituted phenols which could potentially undergo further synthetic manipulation.
Publication status:
Published
Peer review status:
Peer reviewed

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Files:
Publisher copy:
10.1055/s-0035-1561439

Authors


More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Organic Chemistry
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Organic Chemistry
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Organic Chemistry
Role:
Author
More from this funder
Funding agency for:
Frost, J
Donohoe, T
Grant:
EP/L023121/1
EP/L023121/1
Publisher:
Thieme
Journal:
Synthesis More from this journal
Volume:
49
Issue:
4
Pages:
910-916
Publication date:
2016-05-01
Acceptance date:
2016-04-02
DOI:
EISSN:
1437-210X
ISSN:
0039-7881
Keywords:
Pubs id:
pubs:624008
UUID:
uuid:d5a23fac-f11f-4924-9625-4a89b10e4b59
Local pid:
pubs:624008
Source identifiers:
624008
Deposit date:
2016-07-08

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