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Effect of deposited bismuth on the potential of maximum entropy of Pt(111) single-crystal electrodes.

Abstract:

The effect of bismuth adsorption on the entropy of formation of the double layer on Pt(111) electrodes has been studied with the laser-induced temperature jump method. The coulostatic response to the temperature change induced by pulsed laser illumination allows the estimation of the sign and magnitude of the thermal coefficient of the potential drop at the interphase. This is related to the entropy of formation of the double layer, and the particular potential where this thermal coefficient ...

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Publication status:
Published

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Publisher copy:
10.1021/jp061982i

Authors


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Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Physical & Theoretical Chem
Role:
Author
Journal:
journal of physical chemistry. B
Volume:
110
Issue:
42
Pages:
21092-21100
Publication date:
2006-10-01
DOI:
EISSN:
1520-5207
ISSN:
1520-6106
Source identifiers:
40142
Language:
English
Pubs id:
pubs:40142
UUID:
uuid:d47c0867-8340-4212-9a3a-6011ffe92613
Local pid:
pubs:40142
Deposit date:
2012-12-19

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