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Effect of deposited bismuth on the potential of maximum entropy of Pt(111) single-crystal electrodes.

Abstract:

The effect of bismuth adsorption on the entropy of formation of the double layer on Pt(111) electrodes has been studied with the laser-induced temperature jump method. The coulostatic response to the temperature change induced by pulsed laser illumination allows the estimation of the sign and magnitude of the thermal coefficient of the potential drop at the interphase. This is related to the entropy of formation of the double layer, and the particular potential where this thermal coefficient ...

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Publication status:
Published

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Publisher copy:
10.1021/jp061982i

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Institution:
University of Oxford
Department:
Oxford, MPLS, Chemistry, Physical and Theoretical Chem
Role:
Author
Journal:
The journal of physical chemistry. B
Volume:
110
Issue:
42
Pages:
21092-21100
Publication date:
2006-10-05
DOI:
EISSN:
1520-5207
ISSN:
1520-6106
URN:
uuid:d47c0867-8340-4212-9a3a-6011ffe92613
Source identifiers:
40142
Local pid:
pubs:40142
Language:
English

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