Journal article
Fast and selective photoreduction of CO2 to CO Catalyzed by a complex of carbon monoxide dehydrogenase, TiO2, and Ag nanoclusters
- Abstract:
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Selective, visible-light-driven conversion of CO2 to CO with a turnover frequency of 20 s–1 under visible light irradiation at 25 °C is catalyzed by an aqueous colloidal system comprising a pseudoternary complex formed among carbon monoxide dehydrogenase (CODH), silver nanoclusters stabilized by polymethacrylic acid (AgNCs-PMAA), and TiO2 nanoparticles. The photocatalytic assembly, which is stable over several hours and for at least 250000 turnovers of the enzyme’s active site, was investigat...
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- Publication status:
- Published
- Peer review status:
- Peer reviewed
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- Files:
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(Accepted manuscript, pdf, 639.6KB)
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- Publisher copy:
- 10.1021/acscatal.7b04308
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Authors
Funding
+ Royal Society
More from this funder
Funding agency for:
Zhang, L
Grant:
Newton international fellow award (DHR00490
+ Newton Fund
More from this funder
Funding agency for:
Zhang, L
Grant:
Newton international fellow award (DHR00490
+ Biotechnology and Biological Sciences Research Council
More from this funder
Funding agency for:
Armstrong, F
Grant:
BB/M005720/1
Bibliographic Details
- Publisher:
- American Chemical Society Publisher's website
- Journal:
- ACS Catalysis Journal website
- Volume:
- 8
- Issue:
- 4
- Pages:
- 2789−2795
- Publication date:
- 2018-02-27
- Acceptance date:
- 2018-02-15
- DOI:
- EISSN:
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2155-5435
Item Description
- Keywords:
- Pubs id:
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pubs:830323
- UUID:
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uuid:cf3f7f5d-f583-415b-9241-1d5f25625f84
- Local pid:
- pubs:830323
- Deposit date:
- 2018-03-19
Terms of use
- Copyright holder:
- American Chemical Society
- Copyright date:
- 2018
- Notes:
- Copyright © 2018 American Chemical Society. This is the accepted manuscript version of the article. The final version is available online from American Chemical Society at: https://doi.org/10.1021/acscatal.7b04308
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