- Abstract:
-
Selective, visible-light-driven conversion of CO2 to CO with a turnover frequency of 20 s–1 under visible light irradiation at 25 °C is catalyzed by an aqueous colloidal system comprising a pseudoternary complex formed among carbon monoxide dehydrogenase (CODH), silver nanoclusters stabilized by polymethacrylic acid (AgNCs-PMAA), and TiO2 nanoparticles. The photocatalytic assembly, which is stable over several hours and for at least 250000 turnovers of the enzyme’s active site, was investigat...
Expand abstract - Publication status:
- Published
- Peer review status:
- Peer reviewed
- Version:
- Accepted Manuscript
- Files:
-
-
(pdf, 639.6KB)
-
- Publisher copy:
- 10.1021/acscatal.7b04308
-
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- Funding agency for:
- Armstrong, FA
- Publisher:
- American Chemical Society Publisher's website
- Journal:
- ACS Catalysis Journal website
- Volume:
- 8
- Issue:
- 4
- Pages:
- 2789−2795
- Publication date:
- 2018-02-27
- Acceptance date:
- 2018-02-15
- DOI:
- EISSN:
-
2155-5435
- Pubs id:
-
pubs:830323
- URN:
-
uri:cf3f7f5d-f583-415b-9241-1d5f25625f84
- UUID:
-
uuid:cf3f7f5d-f583-415b-9241-1d5f25625f84
- Local pid:
- pubs:830323
- Copyright holder:
- American Chemical Society
- Copyright date:
- 2018
- Notes:
-
Copyright © 2018 American Chemical Society. This is the accepted manuscript version of the article. The final version is available online from American Chemical Society at: https://doi.org/10.1021/acscatal.7b04308
Journal article
Fast and selective photoreduction of CO2 to CO Catalyzed by a complex of carbon monoxide dehydrogenase, TiO2, and Ag nanoclusters
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+ Biotechnology and Biological Sciences Research Council
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