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Inverse modelling of Köhler theory – Part 1: A response surface analysis of CCN spectra with respect to surface-active organic species

Abstract:

In this study a novel framework for inverse modelling of cloud condensation nuclei (CCN) spectra is developed using Köhler theory. The framework is established by using model-generated synthetic measurements as calibration data for a parametric sensitivity analysis. Assessment of the relative importance of aerosol physicochemical parameters, while accounting for bulk–surface partitioning of surface-active organic species, is carried out over a range of atmospherically relevant supersaturation...

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Publication status:
Published
Peer review status:
Peer reviewed
Version:
Publisher's version

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Publisher copy:
10.5194/acp-16-10941-2016

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Department:
Oxford, MPLS, Physics, Atmos Ocean & Planet Physics
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Department:
Oxford, MPLS, Physics, Atmos Ocean & Planet Physics
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Department:
Oxford, MPLS, Physics, Atmos Ocean & Planet Physics
Topping, D More by this author
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Funding agency for:
Stier, Philip
Publisher:
Copernicus Publications Publisher's website
Journal:
Atmospheric Chemistry and Physics Journal website
Publication date:
2016-09-06
Acceptance date:
2016-07-25
DOI:
EISSN:
1680-7324
ISSN:
1680-7316
Pubs id:
pubs:641586
URN:
uri:cedb2f92-6b1e-4b94-b75a-e090d0084cfc
UUID:
uuid:cedb2f92-6b1e-4b94-b75a-e090d0084cfc
Local pid:
pubs:641586

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