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New coordination modes for modified Schiff base Ti(IV) complexes and their control over lactone ring-opening polymerization activity

Abstract:

A series of eight new bis(alkoxy)bis(phenoxy-imine)titanium(IV) catalysts, coordinated by Schiff base ligands derived from o-vanillin (2-hydroxy-3-methoxybenzaldehyde), show good activity and control for the ring-opening polymerization of ε-caprolactone and ω-pentadecalactone. The new complexes are easily prepared in two high-yield steps from commercial reagents. The new ligands can all adopt two different coordination modes, depending on the steric bulk on the imine: a six-membered N–O chela...

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Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1021/acs.inorgchem.8b02271

Authors


More by this author
Institution:
University of Oxford
Division:
MPLS Division
Department:
Chemistry
Sub department:
Inorganic Chemistry
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Oxford college:
Trinity College
Role:
Author
Siam Cement Group (SCG) Chemicals Co., Ltd More from this funder
Publisher:
American Chemical Society Publisher's website
Journal:
Inorganic Chemistry Journal website
Volume:
57
Issue:
22
Pages:
14240–14248
Publication date:
2018-10-30
Acceptance date:
2018-10-11
DOI:
EISSN:
1520-510X
ISSN:
0020-1669
Pubs id:
pubs:926690
UUID:
uuid:ce862ab1-3b90-4494-8d9e-b124c69b334e
Local pid:
pubs:926690
Source identifiers:
926690
Deposit date:
2018-10-11

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