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Journal article

Dual doping effects (site blockage and electronic promotion) imposed by adatoms on Pd nanocrystals for catalytic hydrogen production.

Abstract:
Three distinctive doping effects to modify the electronic and geometric properties of Pd nanocrystals for HCOOH decomposition to H2/CO2 are presented: Bi atoms take preferable residence on higher index sites, which leads to a reduction in HCOOH dehydration; Te atoms dwell favourably on terrace sites, which reduces the rate of dehydrogenation; Ag atoms, without site specificity, induce strong electronic effects to promote the activity on the dwindling number of surface Pd sites at high coverage.
Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1039/c4cc06195k

Authors


Publisher:
Royal Society of Chemistry Publisher's website
Journal:
Chemical Communications Journal website
Volume:
51
Issue:
1
Pages:
46-49
Publication date:
2015-01-01
DOI:
EISSN:
1364-548X
ISSN:
1359-7345
Language:
English
Pubs id:
pubs:485489
UUID:
uuid:c996446c-7f7a-4f98-8020-902138fe7870
Local pid:
pubs:485489
Source identifiers:
485489
Deposit date:
2014-10-04

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