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Nanoparticle surface coverage controls the speciation of electrochemically generated chlorine

Abstract:

Cyclic voltammetry is used to investigate the oxidation of chloride on platinum nanoparticles. The electrochemical response of the nanoparticles dropcast on to a glassy carbon electrode is compared to that recorded at a platinum macroelectrode. The use of ‘nano’ and ‘macro’ scale Pt reveals different ratios of the electrochemically formed products, chlorine (Cl2) and the trichloride (Cl3-) anion. This difference in the speciation is attributed to the chloride oxidation being a surface reactio...

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Publication status:
Published
Peer review status:
Peer reviewed
Version:
Accepted manuscript

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Publisher copy:
10.1002/celc.201600449

Authors


Kraikaew, P More by this author
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Department:
Oxford, MPLS, Chemistry, Physical & Theoretical Chem
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Department:
Oxford, MPLS, Chemistry, Physical & Theoretical Chem
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Department:
Oxford, MPLS, Chemistry, Physical & Theoretical Chem
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Department:
Oxford, MPLS, Materials
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Funding agency for:
Tanner, EEL
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Funding agency for:
Tanner, EEL
Royal Thai Government More from this funder
Publisher:
Wiley Publisher's website
Journal:
ChemElectroChem Journal website
Volume:
3
Issue:
11
Pages:
1794–1798
Publication date:
2016-09-15
Acceptance date:
2016-09-09
DOI:
ISSN:
2196-0216
Pubs id:
pubs:648341
URN:
uri:c8fb9ddc-6aca-417a-8177-6a4026a09b8b
UUID:
uuid:c8fb9ddc-6aca-417a-8177-6a4026a09b8b
Local pid:
pubs:648341
Keywords:

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