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Laplace transform methods for transient diffusion; or, some good questions from Ralph White

Abstract:
Motivated by years of correspondence with Prof. Ralph White, I discuss two unconventional ways to solve diffusion problems with Laplace transforms. A method to derive error-function series, alternatives to Fourier series that converge rapidly and avoid the Gibbs phenomenon at short times, is illustrated by example. It is shown how Mittag-Leffler partial-fractions expansions can facilitate derivations of Fourier-series solutions from the same starting point. Several basic problems pertinent to electrochemical transport are analyzed, culminating in the development of a modified Cottrell equation applicable to thin films of unsupported electrolytic solutions sandwiched between planar electrodes.
Publication status:
Published
Peer review status:
Peer reviewed

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Files:
Publisher copy:
10.1149/1945-7111/acf6e2

Authors


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Institution:
University of Oxford
Division:
MPLS
Department:
Engineering Science
Oxford college:
St Peter's College
Role:
Author
ORCID:
0000-0002-9894-5023


Publisher:
IOP Publishing
Journal:
Journal of The Electrochemical Society More from this journal
Volume:
170
Issue:
9
Article number:
093509
Publication date:
2023-09-20
Acceptance date:
2023-09-05
DOI:
EISSN:
1945-7111
ISSN:
0013-4651


Language:
English
Keywords:
Pubs id:
1526274
Local pid:
pubs:1526274
Deposit date:
2023-09-19

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