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Evaluation of the molecular poisoning phenomenon of W sites in ZSM-5 via synchrotron X-ray powder diffraction

Abstract:
The traditional investigation of complex catalyst poisoning phenomena is in the operation level: poisonings commonly attributed to macroscopic coke deposition and particle size change, etc. Here, we demonstrate that high-resolution SXRD can reveal the structure of the organic molecule–active site complex in a 3-D environment, leading to an understanding of the poisoning mechanism at the molecular level.
Publication status:
Published
Peer review status:
Peer reviewed
Version:
Accepted Manuscript

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Publisher copy:
10.1039/c8cc02904k

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Institution:
University of Oxford
Division:
MPLS Division
Department:
Chemistry
Subgroup:
Inorganic Chemistry
More by this author
Institution:
University of Oxford
Division:
MPLS Division
Department:
Chemistry
Subgroup:
Inorganic Chemistry
More by this author
Institution:
University of Oxford
Division:
MPLS Division
Department:
Chemistry
Subgroup:
Inorganic Chemistry
More by this author
Institution:
University of Oxford
Division:
MPLS Division
Department:
Chemistry
Subgroup:
Inorganic Chemistry
Expand authors...
Publisher:
Royal Society of Chemistry Publisher's website
Journal:
Chemical Communications Journal website
Volume:
54
Issue:
51
Pages:
7014-7017
Publication date:
2018-05-30
Acceptance date:
2018-05-30
DOI:
EISSN:
1364-548X
ISSN:
1359-7345
Pubs id:
pubs:857569
URN:
uri:c0d1fc93-e4fe-458f-8501-160e7511a1c7
UUID:
uuid:c0d1fc93-e4fe-458f-8501-160e7511a1c7
Local pid:
pubs:857569
Language:
English

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