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Product state resolved stereodynamics: Rotational polarization of OH(2II;v′,N′,Ω,f) scattered from the reaction, H+CO2→OH+CO

Abstract:

The quantum state resolved rotational angular momentum alignments of the OH products of the H+CO2 reaction have been determined for a range of states spanning those most populated by reaction at a collision energy of 2.5 eV. Surprisingly, for all quantum states studied, the angular momentum is shown to be aligned preferentially in the scattering plane, containing the reagent and product relative velocity vectors. The data suggest that out-of-plane HO-CO torsional forces play a significant rol...

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Authors


Brouard, M More by this author
Hughes, DW More by this author
Kalogerakis, KS More by this author
Simons, JP More by this author
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Journal:
Journal of Chemical Physics
Volume:
113
Issue:
8
Pages:
3173-3180
Publication date:
2000-08-22
ISSN:
0021-9606
URN:
uuid:bc62a536-5e9a-4046-a1a9-c7b619e6c154
Source identifiers:
151357
Local pid:
pubs:151357
Language:
English

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