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Acoustic phonons and negative thermal expansion in MOF-5.

Abstract:
The mechanism of negative thermal expansion (NTE) in MOF-5 has been studied using a rigid unit mode analysis of the phonons responsible for NTE. In addition to confirming the role of the previously proposed optic 'trampoline mode' mechanism [Lock et al., Dalton Trans., 2013, 42, 1933-2320], we have identified a new acoustic mode mechanism that makes a major contribution to the macroscopic NTE of this framework.
Publication status:
Published

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Publisher copy:
10.1039/c4cp01701c
Publisher:
Royal Society of Chemistry
Journal:
Physical chemistry chemical physics : PCCP
Volume:
16
Issue:
39
Pages:
21144-21152
Publication date:
2014-10-01
DOI:
EISSN:
1463-9084
ISSN:
1463-9076
Language:
English
Pubs id:
pubs:480082
UUID:
uuid:a9d1c77c-8677-4203-86d5-f09717711285
Local pid:
pubs:480082
Source identifiers:
480082
Deposit date:
2014-08-17

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