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Pump and probe spectroscopy with continuous wave quantum cascade lasers.

Abstract:

This paper details infra-red pump and probe studies on nitric oxide conducted with two continuous wave quantum cascade lasers both operating around 5 μm. The pump laser prepares a velocity selected population in a chosen rotational quantum state of the v = 1 level which is subsequently probed using a second laser tuned to a rotational transition within the v = 2 ← v = 1 hot band. The rapid frequency scan of the probe (with respect to the molecular collision rate) in combination with the veloc...

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Publication status:
Published

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Publisher copy:
10.1063/1.4864001
Journal:
Journal of chemical physics
Volume:
140
Issue:
5
Pages:
054311
Publication date:
2014-02-01
DOI:
EISSN:
1089-7690
ISSN:
0021-9606
Language:
English
Pubs id:
pubs:448186
UUID:
uuid:a8c96b01-4e57-4ce5-bc09-af3b1164c619
Local pid:
pubs:448186
Source identifiers:
448186
Deposit date:
2014-06-17

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