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Journal article

Quantifying the electrocatalytic turnover of vitamin B12-mediated dehalogenation on single soft nanoparticles.

Abstract:
We report the electrocatalytic dehalogenation of trichloroethylene by single soft nanoparticles of VB12 containing droplets, and find that the binding between Co (I), the reduced form of Co (III), and TCE is likely a chemically reversible process and in particular using this model system quantify the turnover number and the kinetics of catalytic reactions at individual single soft nanoparticles in real time.
Publication status:
Published
Peer review status:
Peer reviewed

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Publisher copy:
10.1002/anie.201510394

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Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Physical & Theoretical Chem
Role:
Author
More by this author
Institution:
University of Oxford
Division:
MPLS
Department:
Chemistry
Sub department:
Physical & Theoretical Chem
Role:
Author
Publisher:
Wiley Publisher's website
Journal:
Angewandte Chemie (International ed. in English) Journal website
Volume:
55
Issue:
7
Pages:
2545-2549
Publication date:
2016-01-25
Acceptance date:
2015-12-01
DOI:
EISSN:
1521-3773
ISSN:
1433-7851
Language:
English
Keywords:
Pubs id:
pubs:597989
UUID:
uuid:a855cbef-de6d-4dfd-9a71-730395e68f9a
Local pid:
pubs:597989
Source identifiers:
597989
Deposit date:
2016-04-01

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